2o16年中国全国县级科协先进单位个人

来源：蜘蛛抓取(WebSpider) 时间：2016-09-21 01:10 标签： 科协系统先进集体公示
中国科学技术协会var searchResultHtml=$("#tabSearchResult").html();
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题名: Transient response study of NO reduction with H-2 on Co4N/gamma-Al2O3 catalyst
作者: 1,2;
卷号: 109, 期号:2, 页码:461-473关键词:
英文摘要: The reduction of NO with H-2 was studied with transient response experiments on a Co4N/gamma-Al2O3 catalyst. In 1 % NO/1 % H-2/He step-response on Co4N/gamma-Al2O3 catalyst at 300 A degrees C, there were three main stages, viz. initial state, steady state and deactivated state. NO reduction with H-2 generated N-2 and H2O as the main products and NH3 as the by-product during the steady state. Deactivation of the Co4N/gamma-Al2O3 catalyst was due to heavy accumulation of oxygen on the surface. In order to retain a steady-state NO dissociation, the formation of H2O on the catalyst surface was the most crucial step for the removal of surface oxygen, this depended on the NO:H-2 ratio and the reaction temperature. The results indicated that a NO:H-2 ratio of 1:5 and a reaction temperature of 600 A degrees C was determined to keep the Co4N/gamma-Al2O3 catalyst surface sites active for catalytic reduction of NO. Based on the experimental results, the mechanism of reduction of NO with H-2 on Co4N/gamma-Al2O3 catalyst was proposed.
WOS标题词: Science & Technology
Physical Sciences
类目[WOS]: Chemistry, Physical
研究领域[WOS]: Chemistry
关键词[WOS]: NITRIDES
DECOMPOSITION
DISSOCIATION
语种: 英语
WOS记录号:
Citation statistics:
URI标识: []&&
Appears in Collections:
作者单位: 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China2.Dalian Univ Technol, Dalian 116024, Peoples R China
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